For mixed nodes such as Archer+Saber I think of LAlter, maybe Li Shuwen could work too, being arts and evil and both being ST and having defense downs, the damage could be nice on some boss.
On quests with pure sabers, Atalante could be useful to give him the crits and the extra stars for his battery, too, while also boosting the high AOE damage Atalante provides for wave clear.
Also an interesting comp would be coupling him with someone like Ibaraki-Douji. The overall damage is just huge with her demonic nature of Oni.
Medb can also work out as some sub-dps or semi-support, specially against male enemies which aren't uncommon at all. Both get extra bonus with Evil and Male trait, and Medb can also help stall and control male bossess.
Some servants that also could work very nicely with him are the most commons Star Generators Assassins. In fact, pretty much all of them have Evil Alignment (CA Hassan, Shuten Douji, Kotarou, Kojirou, Jack, maybe even Sanson with his triple quick)
I would also consider Vlad III, too, but while the skills aren't bad between themselves, they make use of different supports and utilites, and you just have plain better options than Moriarty as a sub Support, and Vlad as DPS.
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